Chlorine Treatment at Montreal

Source of Supply.Alka-
linity.
Colour.Oxygen
Absorbed
(30 mins.)
Chlorine
Required
p.p.m.
Bacteria
per
c.cm.
Per
Cent
Removed.
Ottawa river15-2050-7014.01.503,000over 98
St. Lawrence river90-100Nil.0.300.30500over 99

Ellms[7] obtained similar results and reported “that the rate at which sterilisation proceeds varies, in a general way, directly with the concentration of the applied available chlorine and the temperature, and inversely as the amount of easily oxidisable matter present.”

Experience with filter plants shows the same facts, the amount of chlorine required for the sterilisation of a filter effluent being invariably less than that necessary to purify the raw water to the same extent.

The effect of coloured organic matter upon the absorption of chlorine, in the form of hypochlorite, is shown on [Diagram I].

DIAGRAM I
EFFECT OF COLOUR ON ABSORPTION OF CHLORINE BY WATER

Absorption of Chlorine
by water at 63° F.
Value of K calculated from
K = Log (N1/N2)When t1 = 0
t2 - t1
Time of
Contact
in
Minutes
Colour of WaterTime of
Contact
in
Minutes
Colour
3254032540
Nil10.0010.0010.00
59.627.706.5050.00330.02270.0374
109.417.035.91100.00260.01530.0228
209.176.405.18200.00180.00960.0190
408.955.824.47400.00120.00570.0087
608.855.633.90600.00080.00410.0068
808.805.583.65800.00070.00320.0056

The shape of the curve obtained with a colour of 40 p.p.m. somewhat resembled that of a mono-molecular reaction and the results were calculated accordingly. The mathematical expression of this law is dN/dt = KN where N is the concentration of the available chlorine in parts per million. Integrating between t1 and t2 the formula K = log(N1/N2)/(t2 - t1) is obtained. If the compound absorbing the chlorine were simple in character, and the chlorine were present in large excess, the value of K would be constant. In the experiments recorded, K constantly decreases, due to the decreasing concentrations of the reacting substances and the complex nature of the organic matter.

The results show the effect of organic matter on the reduction of the chlorine concentration available for germicidal action and also the importance of avoiding a local excess of chlorine (vide [p. 41]).

An effort has been made by some observers to find a quantitative relation between the organic matter, expressed as oxygen absorbed in parts per million, and the chlorine required for oxidation, but without definite result. Some of the results obtained are given in [Table VII].